Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse

Takahashi, Hozumi; Kono, Tatsuya; Sawada, Kosuke; Kumano, Satoru; Tsuri, Yuka; Maruyama, Mihoko; Yoshimura, Masashi; Takahashi, Daisuke; Kawamura, Yukio; Uemura, Matsuo; Nakabayashi, Seiichiro; Mori, Yusuke; Hosokawa, Yoichiroh; Yoshikawa, Hiroshi Y.

doi:https://doi.org/10.1021/acs.jpclett.3c00414

Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse

Takahashi, Hozumi; Kono, Tatsuya; Sawada, Kosuke et al.

Journal of Physical Chemistry Letters, 2023, 14(19), 4394-4402

アクセス数:2,225件（2025-08-15 07:41 集計）

固定URL: https://hdl.handle.net/11094/93293

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タイトル	Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse
著者	著者名 Takahashi, Hozumi
	著者名 Kono, Tatsuya
	著者名 Sawada, Kosuke
	著者名 Kumano, Satoru
	NRID 1000050973062 1000050973062 著者名 Tsuri, Yuka
	NRID 1000020623903 1000020623903 ORCID 0000-0002-3453-8007 0000-0002-3453-8007 researchmap permalink marumarumi marumarumi Scopus Author ID 35307485800 35307485800 著者名 Maruyama, Mihoko
	著者名 Yoshimura, Masashi
	NRID 1000060314382 1000060314382 researchmap permalink read0191199 read0191199 Scopus Author ID 7403136552 7403136552 ORCID 0000-0002-0770-1251 0000-0002-0770-1251 著者名 Takahashi, Daisuke
	NRID 1000010400186 1000010400186 著者名 Kawamura, Yukio
	NRID 1000000213398 1000000213398 著者名 Uemura, Matsuo
	NRID 1000070180346 1000070180346 著者名 Nakabayashi, Seiichiro
	NRID 1000090252618 1000090252618 ORCID 0000-0003-2952-7458 0000-0003-2952-7458 researchmap permalink mori_yusuke mori_yusuke Scopus Author ID 7404197134 7404197134 著者名 Mori, Yusuke
	NRID 1000020448088 1000020448088 著者名 Hosokawa, Yoichiroh
	NRID 1000050551173 1000050551173 researchmap permalink read0108058 read0108058 Scopus Author ID 55708129100 55708129100 ORCID 0000-0003-0624-6039 0000-0003-0624-6039 著者名 Yoshikawa, Hiroshi Y.
内容	Takahashi H., Kono T., Sawada K., et al. Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse. Journal of Physical Chemistry Letters, 14(19), 4394-4402, 18 May 2023: © 2023 American Chemical Society. DOI: 10.1021/acs.jpclett.3c00414.
抄録	Focused irradiation with ultrashort laser pulses realized the fine spatiotemporal control of ice crystallization in supercooled water. An effective multiphoton excitation at the laser focus generated shockwaves and bubbles, which acted as an impulse for inducing ice crystal nucleation. The impulse that was localized close to the laser focus and accompanied by a small temperature elevation allowed the precise position control of ice crystallization and its observation with spatiotemporal resolution of micrometers and microseconds using a microscope. To verify the versatility of this laser method, we also applied it using various aqueous systems (e.g., plant extracts). The systematic study of crystallization probability revealed that laser-induced cavitation bubbles play a crucial role in inducing ice crystal nucleation. This method can be used as a tool for studying ice crystallization dynamics in various natural and biological phenomena.
出版者	American Chemical Society
収録物名	Journal of Physical Chemistry Letters
巻(号)	14(19)
ページ	4394-4402
刊行年月	2023-05-18
言語	英語
ハンドルURL	https://hdl.handle.net/11094/93293
eISSN	19487185
関連情報 (isVersionOf)	DOI (出版社版) https://doi.org/10.1021/acs.jpclett.3c00414
アクセス権	open access
権利情報	This document is the Accepted Manuscript version of a Published Work that appeared in final form in Journal of Physical Chemistry Letters, © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.jpclett.3c00414.
出版タイプ	Accepted Manuscript
カテゴリ	学術雑誌論文 Journal Article

資源タイプ	学術雑誌論文
ローカル資源タイプ	学術雑誌論文
DCMI資源タイプ	text
DCTERMS.bibliographicCitation	Journal of Physical Chemistry Letters. 2023, 14(19), p. 4394-4402
DC.title	Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse
DC.creator	Takahashi, Hozumi
	Kono, Tatsuya
	Sawada, Kosuke
	Kumano, Satoru
	Tsuri, Yuka
	Maruyama, Mihoko
	Yoshimura, Masashi
	Takahashi, Daisuke
	Kawamura, Yukio
	Uemura, Matsuo
	Nakabayashi, Seiichiro
	Mori, Yusuke
	Hosokawa, Yoichiroh
	Yoshikawa, Hiroshi Y.
DC.publisher	American Chemical Society
DC.language' scheme='DCTERMS.RFC1766	英語
DC.type' scheme='DCTERMS.DCMIType	text
DCTERMS.issued' scheme='DCTERMS.W3CDTF	2023-05-18
DC.identifier	https://doi.org/10.1021/acs.jpclett.3c00414
DC.description	Takahashi H., Kono T., Sawada K., et al. Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse. Journal of Physical Chemistry Letters, 14(19), 4394-4402, 18 May 2023: © 2023 American Chemical Society. DOI: 10.1021/acs.jpclett.3c00414.
DCTERMS.abstract	Focused irradiation with ultrashort laser pulses realized the fine spatiotemporal control of ice crystallization in supercooled water. An effective multiphoton excitation at the laser focus generated shockwaves and bubbles, which acted as an impulse for inducing ice crystal nucleation. The impulse that was localized close to the laser focus and accompanied by a small temperature elevation allowed the precise position control of ice crystallization and its observation with spatiotemporal resolution of micrometers and microseconds using a microscope. To verify the versatility of this laser method, we also applied it using various aqueous systems (e.g., plant extracts). The systematic study of crystallization probability revealed that laser-induced cavitation bubbles play a crucial role in inducing ice crystal nucleation. This method can be used as a tool for studying ice crystallization dynamics in various natural and biological phenomena.
DC.rights	This document is the Accepted Manuscript version of a Published Work that appeared in final form in Journal of Physical Chemistry Letters, © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.jpclett.3c00414.
DC.format	93293
citation_title	Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse
citation_author	Takahashi, Hozumi
	Kono, Tatsuya
	Sawada, Kosuke
	Kumano, Satoru
	Tsuri, Yuka
	Maruyama, Mihoko
	Yoshimura, Masashi
	Takahashi, Daisuke
	Kawamura, Yukio
	Uemura, Matsuo
	Nakabayashi, Seiichiro
	Mori, Yusuke
	Hosokawa, Yoichiroh
	Yoshikawa, Hiroshi Y.
citation_publisher	American Chemical Society
citation_language	英語
citation_date	2023-05-18
citation_journal_title	Journal of Physical Chemistry Letters
citation_volume	14
citation_issue	19
citation_firstpage	4394
citation_lastpage	4402
citation_doi	https://doi.org/10.1021/acs.jpclett.3c00414
citation_public_url	https://hdl.handle.net/11094/93293

Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse

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