Design of functional and stable adhesion systems using reversible and movable crosslinked materials

Qian, Yunpeng; Kosaba, Sho; Ikura, Ryohei; Yamaoka, Kenji; Takashima, Yoshinori

doi:https://doi.org/10.1038/s41428-024-01011-7

Design of functional and stable adhesion systems using reversible and movable crosslinked materials

Qian, Yunpeng; Kosaba, Sho; Ikura, Ryohei et al.

Polymer Journal, 2025

Number of Access:514（2025-09-08 07:29 Counts）

Identifier to cite or link to this item: https://hdl.handle.net/11094/100332

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Title	Design of functional and stable adhesion systems using reversible and movable crosslinked materials
Creator	CreatorName Qian, Yunpeng
	CreatorName Kosaba, Sho
	NRID 1000000967565 1000000967565 ORCID 0000-0002-3850-4533 0000-0002-3850-4533 researchmap permalink Ikura-Ryohei Ikura-Ryohei CreatorName Ikura, Ryohei
	ORCID 0000-0001-5655-1643 0000-0001-5655-1643 researchmap permalink yamaokak23 yamaokak23 CreatorName Yamaoka, Kenji
	NRID 1000040379277 1000040379277 ORCID 0000-0002-2620-3266 0000-0002-2620-3266 researchmap permalink ytakashima_0068747 ytakashima_0068747 Scopus Author ID 7103176267 7103176267 CreatorName Takashima, Yoshinori
Description	The version of record of this article, first published in Polymer Journal, is available online at Publisher’s website: https://doi.org/10.1038/s41428-024-01011-7.
Abstract	Stable, tough, and functional adhesion systems are urgently needed for a sustainable society. As a resolution, supramolecular scientists have introduced reversible and movable crosslinked materials into adhesion systems. Reversible crosslinks can repeatedly associate and dissociate. Therefore, reversible crosslinked materials show self-healing and stimuli-responsive properties. Moreover, movable crosslinks are topological crosslinks in which the polymer chains penetrate the cavities of cyclic molecules. The sliding of the movable crosslinks with deformation enabled the achievement of materials showing high toughness and self-relaxation. Adhesion systems with reversible and movable crosslinks have improved adhesion and cohesion, stability, and functionality. This novel concept for the design of adhesion systems is expected to increase the lifetime of adhesives and ameliorate environmental problems.
Publisher	Springer Science and Business Media LLC
Source Title	Polymer Journal
Date of Issued	2025-01-27
Language	English
Handle URL	https://hdl.handle.net/11094/100332
PISSN	00323896
eISSN	13490540
Relation.isIdenticalTo	DOI (Publisher Version) https://doi.org/10.1038/s41428-024-01011-7
Access Rights	open access
CopyRight	This article is licensed under a Creative Commons Attribution 4.0 International License.
oaire:version	Version of Record
Category	学術雑誌論文 Journal Article

Resource Type	journal article
Local Type	Journal Article
DCTERMS.bibliographicCitation	Polymer Journal. 2025
DC.title	Design of functional and stable adhesion systems using reversible and movable crosslinked materials
DC.creator	Qian, Yunpeng
	Kosaba, Sho
	Ikura, Ryohei
	Yamaoka, Kenji
	Takashima, Yoshinori
DC.publisher	Springer Science and Business Media LLC
DC.language' scheme='DCTERMS.RFC1766	English
DCTERMS.issued' scheme='DCTERMS.W3CDTF	2025-01-27
DC.identifier	https://doi.org/10.1038/s41428-024-01011-7
DC.description	The version of record of this article, first published in Polymer Journal, is available online at Publisher’s website: https://doi.org/10.1038/s41428-024-01011-7.
DCTERMS.abstract	Stable, tough, and functional adhesion systems are urgently needed for a sustainable society. As a resolution, supramolecular scientists have introduced reversible and movable crosslinked materials into adhesion systems. Reversible crosslinks can repeatedly associate and dissociate. Therefore, reversible crosslinked materials show self-healing and stimuli-responsive properties. Moreover, movable crosslinks are topological crosslinks in which the polymer chains penetrate the cavities of cyclic molecules. The sliding of the movable crosslinks with deformation enabled the achievement of materials showing high toughness and self-relaxation. Adhesion systems with reversible and movable crosslinks have improved adhesion and cohesion, stability, and functionality. This novel concept for the design of adhesion systems is expected to increase the lifetime of adhesives and ameliorate environmental problems.
DC.rights	This article is licensed under a Creative Commons Attribution 4.0 International License.
DC.format	100332
citation_title	Design of functional and stable adhesion systems using reversible and movable crosslinked materials
citation_author	Qian, Yunpeng
	Kosaba, Sho
	Ikura, Ryohei
	Yamaoka, Kenji
	Takashima, Yoshinori
citation_publisher	Springer Science and Business Media LLC
citation_language	English
citation_date	2025-01-27
citation_journal_title	Polymer Journal
citation_doi	https://doi.org/10.1038/s41428-024-01011-7
citation_public_url	https://hdl.handle.net/11094/100332

Design of functional and stable adhesion systems using reversible and movable crosslinked materials

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