Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse

Takahashi, Hozumi; Kono, Tatsuya; Sawada, Kosuke et al.

Journal of Physical Chemistry Letters, 2023, 14(19), 4394-4402

Number of Access:2,317（2025-09-30 08:03 Counts）

Identifier to cite or link to this item: https://hdl.handle.net/11094/93293

Link to primary information 

File Format Terms of use Size Views Date.Available Description information
JPhysChemLett_14_19_4394 pdf None 1.00 MB 149 2024.05.18  

Item Information

Output File Export EndNote Basic Export Mendeley

Title
Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse
Creator
CreatorName
Takahashi, Hozumi
CreatorName
Kono, Tatsuya
CreatorName
Sawada, Kosuke
CreatorName
Kumano, Satoru
NRID
1000050973062 1000050973062
CreatorName
Tsuri, Yuka
NRID
1000020623903 1000020623903
ORCID
0000-0002-3453-8007 0000-0002-3453-8007
researchmap permalink
marumarumi marumarumi
Scopus Author ID
35307485800 35307485800
CreatorName
Maruyama, Mihoko
CreatorName
Yoshimura, Masashi
NRID
1000060314382 1000060314382
researchmap permalink
read0191199 read0191199
Scopus Author ID
7403136552 7403136552
ORCID
0000-0002-0770-1251 0000-0002-0770-1251
CreatorName
Takahashi, Daisuke
NRID
1000010400186 1000010400186
CreatorName
Kawamura, Yukio
NRID
1000000213398 1000000213398
CreatorName
Uemura, Matsuo
NRID
1000070180346 1000070180346
CreatorName
Nakabayashi, Seiichiro
NRID
1000090252618 1000090252618
ORCID
0000-0003-2952-7458 0000-0003-2952-7458
researchmap permalink
mori_yusuke mori_yusuke
Scopus Author ID
7404197134 7404197134
CreatorName
Mori, Yusuke
NRID
1000020448088 1000020448088
CreatorName
Hosokawa, Yoichiroh
NRID
1000050551173 1000050551173
researchmap permalink
read0108058 read0108058
Scopus Author ID
55708129100 55708129100
ORCID
0000-0003-0624-6039 0000-0003-0624-6039
CreatorName
Yoshikawa, Hiroshi Y.
Description
Takahashi H., Kono T., Sawada K., et al. Spatiotemporal Control of Ice Crystallization in Supercooled Water via an Ultrashort Laser Impulse. Journal of Physical Chemistry Letters, 14(19), 4394-4402, 18 May 2023: © 2023 American Chemical Society. DOI: 10.1021/acs.jpclett.3c00414.
Abstract
Focused irradiation with ultrashort laser pulses realized the fine spatiotemporal control of ice crystallization in supercooled water. An effective multiphoton excitation at the laser focus generated shockwaves and bubbles, which acted as an impulse for inducing ice crystal nucleation. The impulse that was localized close to the laser focus and accompanied by a small temperature elevation allowed the precise position control of ice crystallization and its observation with spatiotemporal resolution of micrometers and microseconds using a microscope. To verify the versatility of this laser method, we also applied it using various aqueous systems (e.g., plant extracts). The systematic study of crystallization probability revealed that laser-induced cavitation bubbles play a crucial role in inducing ice crystal nucleation. This method can be used as a tool for studying ice crystallization dynamics in various natural and biological phenomena.
Publisher
American Chemical Society
Source Title
Journal of Physical Chemistry Letters
Volume (Issue)
14(19)
Page
4394-4402
Date of Issued
2023-05-18
Language
English
Handle URL
https://hdl.handle.net/11094/93293
eISSN
19487185
Relation.isVersionOf
DOI (Publisher Version)
https://doi.org/10.1021/acs.jpclett.3c00414
Access Rights
open access
CopyRight
This document is the Accepted Manuscript version of a Published Work that appeared in final form in Journal of Physical Chemistry Letters, © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.jpclett.3c00414.
oaire:version
Accepted Manuscript
Category
学術雑誌論文 Journal Article